High school student Ageha Yoshina, renowned for his self-assurance, earns a living by aiding others. One fateful day, he stumbles upon a peculiar calling card labeled 'Psyren' in a phone booth and decides to pocket it, oblivious to its significance. Soon after, Ageha learns that his classmate Sakurako Amamiya possesses an identical card, sparking a chain of events as she pleads for his help. As he grapples with the mysteries unfolding around him, Sakurako vanishes, prompting Ageha to dial the card's number and engage with a mysterious entity. This sets in motion a perilous journey for the two teenagers, thrust into a deadly game in an otherworldly realm infested with monstrous beings known as 'Taboo.' Endowed with psychic abilities dubbed 'PSI,' they strive to survive and find a way back to their familiar world.

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